Tensile and viscoelastic characterization of magnetorheological elastomers with varying carbonyl iron particle concentration
-
Published: April 12, 2026
Abstract
Magnetorheological elastomers (MREs) are smart composite materials whose mechanical properties can be tuned under magnetic fields, making them ideal for adaptive vibration control. This study examines the viscoelastic behavior of MREs containing 0%, 10%, 20% 30%, 40% and 50% carbonyl iron particles (CIPs) through uniaxial tensile testing. Key mechanical parameters, including tensile stress at 0.2% strain, modulus, and load at yield, were evaluated across twelve samples. The storage modulus was determined using both Rubber Elasticity Theory and the Maxwell–Kelvin viscoelastic model to compare their predictive accuracy. Results revealed that the storage modulus increased with CIP content up to 30% (1.5 MPa, Rubber Elasticity Theory) before slightly declining at 50% (0.6 MPa), likely due to particle agglomeration. The Rubber Elasticity Theory consistently predicted higher moduli than the Maxwell–Kelvin model. Qualitatively, damping improved with higher CIP content, indicated by greater load at yield. These findings highlight the crucial role of filler concentration in tailoring MRE stiffness and damping performance, while emphasizing the need for dynamic mechanical testing to validate energy dissipation mechanisms. The study provides insights into optimizing MRE formulations for engineering applications such as vibration isolation and adaptive control systems.
- Carbonyl iron particles
- Damping
- Magnetorheological elastomer
- Storage modulus
- Tensile testing

This work is licensed under a Creative Commons Attribution-NonCommercial-ShareAlike 4.0 International License.
- Asadi, H., Khodadadi, M., & Khosravi, H. (2023). Mechanical characterization of isotropic and anisotropic MREs under uniaxial loading. Smart Materials and Structures, 32(2), 025006. https://doi.org/10.1088/1361-665X/acb1a5
- Cheng, M., Li, Y., & Gong, X. (2022). Fabrication and properties of RTV-silicone-based MREs with varied CIP content. Journal of Materials Science, 57(3), 1891–1905. https://doi.org/10.1007/s10853-021-06669-5
- Dargahi, A., Sedaghati, R., & Rakheja, S. (2019). On the properties of magnetorheological elastomers in shear mode: Design, fabrication and characterization. Composites Part B: Engineering, 159, 269–283. https://doi.org/10.1016/j.compositesb.2018.09.080
- Dhakad, R., Hipparkar, D. R., Kumar, A., & Chandel, S. (2023). A hyper-viscoelastic constitutive model for elastomers: A case study of hydrogenated nitrile butadiene rubber and polychloroprene rubber. Journal of Elastomers & Plastics, 55(7), 1013–1034. https://doi.org/10.1177/00952443231191765
- Díez, A. G., Tubio, C. R., Etxebarria, J. G., et al. (2021). Magnetorheological elastomer‐based materials and devices: state of the art and future perspectives. Advanced Engineering Materials, 23(12), 2100240. https://doi.org/10.1002/adem.202100240
- Fan, Y., Gong, X., Xuan, S., & Zhang, W. (2011). Interfacial friction damping properties in magnetorheological elastomers. Smart Materials and Structures, 20(3), 035007. https://doi.org/10.1088/0964-1726/20/3/035007
- Gomez-Color, J. L., Palacios-Pineda, L. M., & Perales, E. (2025). Study on stiffness and damping of magnetorheological elastomers under biaxial loads. Polymer Testing, 128, 107012. https://doi.org/10.1016/j.polymertesting.2024.107012
- Hapipi, N., Mazlan, S. A., Aziz, S. A. A., Ubaidillah, U., Mohamad, N., Yazid, I. I. M., & Choi, S. B. (2018). Effect of curing current on stiffness and damping properties of magnetorheological elastomers. International Journal of Sustainable Transportation Technology, 1(2), 51-58.
- Johari, M. A. F., Mazlan, S. A., Nordin, N. A., & Ubaidillah, U. (2021). The effect of microparticles on the storage modulus and durability behavior of magnetorheological elastomer. Micromachines, 12(8), 948. https://doi.org/10.3390/mi12080948
- Kallio, M. (2005). The elastic and damping properties of magnetorheological elastomers (VTT Publications 565). VTT Technical Research Centre of Finland.
- Khimi, S. R., & Pickering, K. L. (2015). Comparison of dynamic properties of magnetorheological elastomers with existing antivibration rubbers. Composites Part B: Engineering, 83, 175–183. https://doi.org/10.1016/j.compositesb.2015.08.017
- Kim, J., Shin, H., & Park, J. (2025). Advanced MRE composites for adaptive vibration suppression. Composites Science and Technology, 242, 110985. https://doi.org/10.1016/j.compscitech.2025.110985
- Li, D., Zhang, Y., & Chen, Q. (2022). Effect of crosslink density on mechanical and viscoelastic properties of silicone-based MREs. Polymer Testing, 110, 107551. https://doi.org/10.1016/j.polymertesting.2022.107551
- Li, X., Ruan, X., & Li, L. (2023). Theoretical and experimental research on the mechanical properties of magnetorheological elastomers based on PDMS. Frontiers in Materials, 10, 1253055. https://doi.org/10.3389/fmats.2023.1253055
- Liang, Y., Chen, X., & Liu, Z. (2024). Nano-scale dispersion control in silicone-based magneto-elastomers. Polymer Testing, 129, 107022. https://doi.org/10.1016/j.polymertesting.2024.107022
- Lu, Y., Wang, B., & Zang, C. (2023). Analysis of energy dissipation in MREs using yield point indicators. Journal of Intelligent Material Systems and Structures, 34(5), 617–628. https://doi.org/10.1177/1045389X221132190
- Magin, R. L., & Royston, T. J. (2010). Fractional-order elastic models of cartilage: A multi-scale approach. Communications in Nonlinear Science and Numerical Simulation, 15(3), 636–643. https://doi.org/10.1016/j.cnsns.2009.05.008
- Nam, T. H., Petríková, I., & Marvalová, B. (2020). Experimental characterization and viscoelastic modeling of isotropic and anisotropic magnetorheological elastomers. Polymer Testing, 81, 106272. https://doi.org/10.1016/j.polymertesting.2019.106272
- Nam, T. H., Petríková, I., & Marvalová, B. (2022). Effects of loading rate, applied shear strain, and magnetic field on stress relaxation of anisotropic MREs. Mechanics of Advanced Materials and Structures, 29(14), 2614–2624. https://doi.org/10.1080/15376494.2021.1883162
- Norouzi, M., Gilani, M., & Alehashem, S. M. S. (2017). Dynamic characterization and modeling of isotropic magnetorheological elastomers under tensile-compressive loadings. IEEE Transactions on Magnetics, 53(11), 1–9. https://doi.org/10.1109/TMAG.2017.2731398
- Nugroho, K. C. (2024). Influence of carbonyl iron particles on the structural and mechanical performance of magnetorheological elastomers. Multidisciplinary Innovations and Research in Applied Engineering. https://doi.org/10.70935/4v17g706
- Park, J., Choi, Y. T., Flatau, A., & Wereley, N. M. (2022). Encapsulations of magnetorheological fluids within 3-D printed elastomeric cellular structures. IEEE Transactions on Magnetics, 58(6), 1–5. https://doi.org/10.1109/tmag.2021.3137838
- Patel, D., & Upadhyay, R. V. (2023). Fractional Maxwell viscoelastic model to explain dynamic magneto-viscoelastic properties of an isotropic magnetorheological elastomer. Soft Materials, 22(5), 501–510. https://doi.org/10.1080/1539445X.2023.2247002
- Patel, D., Upadhyay, R. V., & Mazlan, S. A. (2024). A modified parametric model to predict visco-elastic properties of magneto-rheological elastomers at non-LVE region. Journal of Intelligent Material Systems and Structures. https://doi.org/10.1177/1045389X241272994
- Pavel, R., Singh, V., & Thomas, A. (2022). Linear viscoelastic modeling of magneto-sensitive elastomers using small-strain uniaxial tests. Mechanics of Materials, 166, 104298. https://doi.org/10.1016/j.mechmat.2022.104298
- Puente-Córdova, J. G., Reyes-Melo, M. E., & Rodríguez, J. A. (2018). Fabrication and characterization of isotropic and anisotropic magnetorheological elastomers. Polymers, 10(12), 1343. https://doi.org/10.3390/polym10121343
- Qiao, Y., Zhang, J., Zhang, M., Liu, L., & Zhai, P. (2021). A magnetic field- and frequency-dependent dynamic shear modulus model for isotropic silicone rubber-based magnetorheological elastomers. Composites Science and Technology, 204, 108637. https://doi.org/10.1016/j.compscitech.2020.108637
- Rosdi, M. A. M., Saad, M., & Sulaiman, N. (2023). Qualitative evaluation of damping in magnetorheological elastomers via static yield tests. Materials Research Express, 10(1), 015701. https://doi.org/10.1088/2053-1591/ac9fb2
- Safaei, B., Jafari, A., & Hemmati, M. (2023). Modeling the storage modulus of filled elastomers via chain network theory. Polymer, 263, 125415. https://doi.org/10.1016/j.polymer.2022.125415
- Salim, N. J., & Matlack, K. H. (2024). Dynamic magneto-mechanical analysis of isotropic and anisotropic magneto-active elastomers. Experimental Mechanics. https://doi.org/10.1007/s11340-024-01115-4
- Singh, R., & Zhang, Y. (2025). Frequency-dependent mechanical tuning in hybrid magnetorheological elastomers under dual-field excitation. Smart Materials and Structures, 34(1), 015004. https://doi.org/10.1088/1361-665X/ad7c19
- Siti Nor, F. H., Md. Isa, M. A., & Azmi, W. H. (2023). Magneto-mechanical behavior of silicone rubber with CIP: A comparative analysis. Results in Physics, 48, 107205. https://doi.org/10.1016/j.rinp.2023.107205
- Soria-Hernández, C. G., Palacios-Pineda, L. M., Elías-Zúñiga, A., Perales-Martínez, I. A., & Martínez-Romero, O. (2019). Investigation of the Effect of Carbonyl Iron Micro-Particles on the Mechanical and Rheological Properties of Isotropic and Anisotropic MREs: Constitutive Magneto-Mechanical Material Model. Polymers, 11(10), 1705. https://doi.org/10.3390/polym11101705
- Sun, T. L., Gong, X. L., Jiang, W. Q., Li, J., & Li, W. (2008). Study on the damping properties of magnetorheological elastomers based on cis‑polybutadiene rubber. Polymer Testing, 27(4), 520–526. https://doi.org/10.1016/j.polymertesting.2008.02.008
- Wan, Y., Xiong, Y., & Zhang, S. (2018). Temperature effect on viscoelastic properties of anisotropic magnetorheological elastomers under compression. Smart Materials and Structures, 27(12), 125014. https://doi.org/10.1088/1361-665X/aaeaf8
- Wang, B., & Kari, L. (2020). A visco-elastic-plastic constitutive model of isotropic magneto-sensitive rubber with amplitude, frequency and magnetic dependency. International Journal of Plasticity, 132, 102756. https://doi.org/10.1016/j.ijplas.2020.102756
- Wang, H., He, Q., & Zhao, Y. (2023). Simplified Maxwell-Kelvin modeling for quasi-static MRE characterization. Journal of Applied Polymer Science, 140(17), e53690. https://doi.org/10.1002/app.53690
- Yaghoobi, A., Jalali, A., & Norouzi, M. (2022). Aspect ratio dependency of magneto-rheological elastomers in dynamic tension-compression loading. IEEE Transactions on Magnetics. https://doi.org/10.1109/TMAG.2022.3146377
- Yang, Y., Liu, X., & Wu, Y. (2022). Viscoelastic performance of MREs under small strain amplitude: Static and dynamic comparisons. Composites Science and Technology, 223, 109445. https://doi.org/10.1016/j.compscitech.2022.109445
- Yarali, E., Farajzadeh, M. A., Noroozi, R., & Dabbagh, A. (2020). Magnetorheological elastomer composites: Modeling and dynamic finite element analysis. Composites Part B: Engineering, 201, 108379. https://doi.org/10.1016/j.compositesb.2020.108379
- Zakaria, A. A. (2024). Smart viscoelastic supports for vibration control in rotors (Doctoral dissertation, University of Southampton).https://eprints.soton.ac.uk/489035
- Zhang, H., Li, A., Su, Y., Xu, G., & Ben, S. (2024). Viscoelastic dampers for civil engineering structures: A systematic review. Journal of Building Engineering, 90, 108019. https://doi.org/10.1016/j.jobe.2024.108019